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Thermophysics and Aeromechanics

2008 year, number 3

Modelling of methanol-to-hydrogen steam reforming with a heat flux distributed along a microchannel

V.V. Kuznetsov1, S.P. Kozlov2
1 Kutateladze Institute of Thermophysics SB RAS, Novosibirsk, Russia Novosibirsk State University, Novosibirsk, Russia, vladkus@itp.nsc.ru
2 Kutateladze Institute of Thermophysics SB RAS, Novosibirsk, Russia Novosibirsk State University, Novosibirsk, Russia
Keywords: methanol steam reforming, heat and mass transfer, chemical transformation, microchannel, catalytic reaction
Pages: 509-517

Abstract

The flow of reacting mixture of methanol and steam in a 2D microslot was studied numerically at activation of the reactions on the channel wall. This modelling was carried out in the framework of Navier - Stokes equations for a laminar flow of multicomponent compressible gas. Correlations between thermal, diffusion, and physical-chemical processes were studied under the conditions of intense endothermic reaction and external heat supply distributed along the channel. It is shown that not only the amount of heat supplied to the reaction zone is essential, but also the mode of heat supply along the channel length is important, which allows optimization of the compact reactor for hydrogen production.